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And Kersting, B. (2007) Synthesis, 3706–3712. Gressenbuch, M. D. Thesis, Universit€at Leipzig. Siedle, G. and Kersting, B. (2003) Zeitschrift fur Anorganische und Allgemeine Chemie, 629, 2083–2090. Gressenbuch, M. and Kersting, B. (2007) European Journal of Inorganic Chemistry, 90–102. , McMaster, J. and Schr€oder, M. (2003) Chemical Communications, 1098–1099. Brooker, S. (2001) Coordination Chemistry Reviews, 222, 33–56. , Lozan, V. and Kersting, B. (2006) Dalton Transactions, 1738–1748. Lozan, V.

Reactivity is relevant as end-on copper complexes play a role in nature’s enzymatic CH hydroxylation reactions. At the same time, when we proposed the existence of this end-on superoxo complex, Prigge et al. presented an unusual end-on Cu-O2 complex observed in an XRD structure of pepdidylglycine-a-hydroxylating monooxygenase [33] refined to 185 pm. This important finding supports the view that an end-on superoxo mono copper site is the precatalytic species in the a-hydroxylation of CÀH bonds by this enzyme.

2005) Angewandte Chemie – International Edition, 44, 1000–1002. , Tamura, M. and Fujita, M. (2006) Science, 312, 251–254. , Hori, A. and Therrrien, B. (2005) Accounts of Chemical Research, 38, 371–398. W. C. (1997) Progress in Inorganic Chemistry, 45, 1–83. Armspach, D. and Matt, D. (1999) Chemical Communications, 1073–1074. J. A. (1997) Inorganic Chemistry, 36, 5498–5504. J. N. (2000) Chemical Society Reviews, 29, 75–86. T. R. (1997) Angewandte Chemie (International Edition in English), 36, 865–867.

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