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Extra info for Activating Unreactive Substrates The Role of Secondary Interactions
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Reactivity is relevant as end-on copper complexes play a role in natures enzymatic CH hydroxylation reactions. At the same time, when we proposed the existence of this end-on superoxo complex, Prigge et al. presented an unusual end-on Cu-O2 complex observed in an XRD structure of pepdidylglycine-a-hydroxylating monooxygenase  reﬁned to 185 pm. This important ﬁnding supports the view that an end-on superoxo mono copper site is the precatalytic species in the a-hydroxylation of CÀH bonds by this enzyme.
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